To seal a joint which opens up during dynamic load cycles will require a gasket with enough flexibility to retain a seal.
As I have repeatedly stated the problem of introducing a gasket between the joint faces is that it greatly reduces the fatigue strength of the bolt. This reduces the load capacity of the axle. I have only done some quick mental arithmetic, but expect it to be "in the ball park", which indicates that portal axles bolted to stock axle tubes reduce the load capacity of the front axle to about 60 or 70% of a stock defender axle. This capacity reduction assumes that the bolts are pre-loaded sufficiently to prevent the joint opening. If the pre-load is not sufficient then the load capacity needs to be reduced even further so that the pre-load will prevent the joint opening.
Besides the greater moment and torsional shear loads during braking due to the increased offset and weight, portals impose additional load cycles upon the bolts that the stock axle does not have - torque reactions from stock half-shafts are transferred through the diff housing to the inner section of the axle tubes to the radius arms, but the portal box transferes the torque reaction through the swivel ball and bolted joint, into the outer ends of the axle tubes to the radius arms. When the bolts are already overloaded the last thing they need is thousands of additional load cycles reducing their life.
IMHO, oil leaking is a problem, but it is not the important problem here and no attempt to prevent oil leak should compromise the strength of these bolts. If they break on the Simpson crossing (which is a lot more severe from anything that I gather has been encounted so far), then a gasket won't prevent the diff or portal box from filling with sand while the truck is dragged back down a dune.
The svivel ball has a spigot that locates in a recess inside the flange on the end of the axle tube. There is a chamfer in the corner of the recess.
An O-ring could work if you obtained one of the correct section and inside diameter to fit into the space between the small fillet radius at the swivel ball spigot and the chamfer in the axle tube recess. Then you still have a metal to metal joint.
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