As our friend from the RTA says "You can in fact do anything" they just don't have to register it.
The problem is that the 1972 engine will have to pass 1986 emission control regs as specified in the ADR's. Which basically means that all the fittings from the 1986 engine need to go back on the 1972 engine. Then yes you can EFI the 1972 engine.
Another issue you may wish to consider, aluminium blocks crystalise over time and will therefore be more prone to cracks. The early 3.5 engines are not as strong in the block as the later engines, like your original 1986 block.
Thirdly, a 1972 is a very early Range Rover engine, in restorable condition the 1972 donor is potentially more valuable than the 1986.
Hope this helps.
Regards
Diana


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