IMO you should make a test with stock tyres before a final conclusion, with those huge tyres the whole addaptive strategy of the management might be mixed up as long as the new fuel map was not especially conceived for that by someone who really knows his stuff cos there's a missmatch now it the ECM's "brain" as with those tyres the VSS(vehicle speed signal, part of the addaptive strategy) is unexpectedly low according to the revs and torque delivered at a certain vehicle speed and the fuel map was ''calibrated"" for stock(or max 5% greater) tyres, as your's is manual there's no default value for VSS(only autos have it) so the management will compensate by overfueling.
IMO for those tyres you need dedicated fuel map to not have any issues also if i understood well you dont even have a larger intercooler yet which is not healthy with any remap
can't you take a live data log with a nanocom to see some MAF, MAP, IAT values?
Discovery Td5 (2000), manual, tuned
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